| 1 | –Percy Faith | Exodus |
| 2 | –Tony Bennett | I Wanna Be Aound |
| 3 | –Gene Pitney | Only Love Can Break A Heart |
| 4 | –Ray Conniff | Invisible Tears |
| 5 | –Bobby Vinton | Roses Are Red (My Love) |
| 6 | –Terry Baxter | Alfie |
| 7 | –Robert Goulet | My Love Forgive Me |
| 8 | –David Houston | Almost Persaded |
| 9 | –Paul Mauriat | Love Is Blue |
| 10 | –Percy Faith | Theme From "A Summer Place" |
| 11 | –Steve Lawrence | Go Away Little Girl |
| 12 | –Lulu | To Sir With Love |
| 13 | Greatest Love Songs Of The Sensational 60s |
| 14 | –Jim Nabors | The Impossible Dream |
| 15 | –The New Christy Minstrels | Chim, Chim, Cher-ee |
| 16 | –John Davidson | A Taste Of Honey |
| 17 | –Connie Francis | Everybody's Somebody's Fool |
| 18 | –The Statler Brothers | Flowers On The Wall |
| 19 | –Unknown Artist | Lara's Theme (Original Soundtrack) |
| 20 | –Johnny Mathis | Love Theme From "Romeo And Juliet" |
| 21 | –Patti Page | Hush, Hush, Sweet Charlotte |
| 22 | Great Hits From The Sensational 60s |
| 23 | –John Barry | Born Free |
| 24 | –Marty Robbins | Devil Woman |
| 25 | –Connie Francis | Where The Boys Are |
| 26 | –Jim Nabors | What Now My Love |